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Sn元素对均匀态Mg-6Zn-0.25Ca镁合金耐腐蚀性能影响的研究
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1.沈阳化工大学 机械与动力工程学院;2.沈阳大学机械工程学院

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国家自然基金青年科学基金(52201131);辽宁省科技厅自然基金(2022-MS-253)


The research investigates the impact of Sn element on the corrosion resistance of a homogenized Mg-6Zn-0.25Ca magnesium alloy
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    摘要:

    研究了添加1%的Sn对均匀态Mg-6Zn-0.25Ca合金耐腐蚀性能的影响。通过OM、XRD、SEM、析氢失重以及极化曲线实验来分析Mg-6Zn-Sn-0.25Ca(1k)以及Mg-6Zn-0.25Ca(10k)两种合金的耐腐蚀性能。结果表明,Mg-6Zn-0.25Ca(10k)合金主要第二相是Mg2Ca相,再加入Sn元素后,Mg-6Zn-Sn-0.25Ca合金中第二相的主要存在方式为Mg2Sn相、Mg2Ca相和少量CaMgSn相。加入Sn元素增强了Mg-6Zn-0.25Ca合金的耐蚀能力,加入Sn元素后,合金第二相分布更加均匀,合金的平均晶粒尺寸由145.6um下降到了114.2um,因为高熔点的Mg2Sn相可以作为α-Mg基体非自发结晶的异质形核核心,从而细化晶粒尺寸。在两者共同作用下,合金因腐蚀而产生的氧化膜更加绵密,阻止了析氢反应的继续进行。此外,极化曲线表明,Mg-6Zn-0.25Ca合金的自腐蚀电位和自腐蚀电流密度分别为-1.729V和2.106×10-5μA/cm2,添加1%Sn元素后,自腐蚀电位升高到-1.525V,自腐蚀电流密度减小为8.561×10-6μA/cm2,增强了Mg-6Zn-Sn-0.25Ca合金的耐蚀能力。

    Abstract:

    The effect of adding 1% Sn on the corrosion resistance of homogeneous Mg-6Zn-0.25Ca alloy was studied. The corrosion resistance of Mg-6Zn-Sn-0.25Ca(1k) and Mg-6Zn-0.25Ca(10k) alloys was analyzed by OM, XRD, SEM, hydrogen evolution weight loss and polarization curve experiments. The results show that the main second phase of Mg-6Zn-0.25Ca(10k) alloy is Mg2Ca phase, and after the addition of Sn element, the main mode of existence of the second phase in Mg-6Zn-Sn-0.25Ca alloy is Mg2Sn phase, Mg2Ca phase and a small amount of CaMgSn phase. The addition of Sn element enhances the corrosion resistance of Mg-6Zn-0.25Ca alloy, and the second phase of the alloy is more evenly distributed after the addition of Sn element, and the average grain size of the alloy decreases from 145.6um to 114.2um, because the Mg2Sn phase with high melting point can be used as a heterogeneous nucleation core for non-spontaneous crystallization of the α-Mg matrix, thereby refining the grain size. Under the combined effect of the two, the oxide film produced by the corrosion of the alloy is more dense, preventing the hydrogen evolution reaction from proceeding. In addition, the polarization curves show that the self-corrosion potential and self-corrosion current density of Mg-6Zn-0.25Ca alloy are -1.729V and 2.106×10-5 μA/cm2, respectively, and the self-corrosion potential increases to -1.525V and the self-corrosion current density decreases to 8.561×10-6μA/cm2, which enhances the corrosion resistance of Mg-6Zn-Sn-0.25Ca alloy.

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郭树国,刘绪栋,贾征,寇荣辉,刘全. Sn元素对均匀态Mg-6Zn-0.25Ca镁合金耐腐蚀性能影响的研究[J].稀有金属材料与工程,,().[guoshuguo, liuxudong, jiazheng, kouronghui, liuquan. The research investigates the impact of Sn element on the corrosion resistance of a homogenized Mg-6Zn-0.25Ca magnesium alloy[J]. Rare Metal Materials and Engineering,,().]
DOI:10.12442/j. issn.1002-185X.20240160

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  • 收稿日期:2024-03-20
  • 最后修改日期:2024-04-28
  • 录用日期:2024-05-08
  • 在线发布日期: 2024-06-17
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